I think so, I think Ocarina of Time earns its high esteem, and Ship of Harkinian irons out a lot of the QoL issues that make the original annoying, like being able to toggle boots without going into the menu.

After you finish OoT I’d recommend running Majora’s Mask via 2 Ship 2 Harkinian as well. It’s less popular than OoT but every bit as good, I think. I can’t pick just one, but if I had to pick a “#1 favorite video game of all time”, Majora’s Mask would be a finalist. It’s really good.